The structure that is least likely to exist is HS.
Sulfur is an element in group 16. Sulfur is a divalent element that has two lone pairs of electrons. This means that sulfur forms compounds in which it is bonded to two atoms or groups.
All the molecules listed can exist because they consists of structures in which sulfur is bonded to two atoms or groups. The only structure that can not exist is HS because it does not satisfy the valency of sulfur.
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